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Shaomingfei

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Introduction

Mingfei Shao received his Ph.D. degree from Beijing University of Chemical Technology (BUCT) in 2014, after which he joined the staff of BUCT and was promoted to professor in 2018. He was also a visiting student at the University of Oxford in 2013. His research interests include intercalation chemistry and energy materials, electrocatalysis/photoelectrocatalysis and advanced energy devices. He proposed the idea of the water electrolysis coupled with green electrosynthesis (e.g., hydrogen generation coupled with organic oxidation). He also proposed a new method of integrated electrode design based on layered double hydroxides, which is a platform for construct various energy materials and devices. He has been published more than 110 papers, which have been cited >14,000 times (H index= 65). In addition, He has obtained and awarded from the National Natural Science Foundation of China–Outstanding Youth Foundation in 2019 and the Chinese Catalytic Rookie Award

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Publications

1. Yining Sun, Kui Fan, Jinze Li, Zhenhua Li*, Mingfei Shao* and Xue Duan, Boosting Electrochemical Oxygen Reduction to Hydrogen Peroxide by Efficient Electrocatalyst and Coupled with Organic Oxidation, Nat. Commun. 2024, 15, 6098.

2. Kui Fan, Wenfu Xie, Jinze Li, Yining Sun, Pengcheng Xu, Yang Tang, Zhenhua Li, Mingfei Shao*, Active hydrogen boosts electrochemical nitrate reduction to ammonia Nat. Commun. 2022, 13, 7958

3. Jiangrong Yang, Tian Xia, Hao Li, Hong Yan, Xianggui Kong, Zhenhua Li, Mingfei Shao, Xue Duan, Evaluation of Active Oxygen Species Derived from Water Splitting for Electrocatalytic Organic Oxidation, Angew. Chem. Int. Ed. 2024, e202413457

4. Zhenhua Li, Haohong Duan, Mingfei Shao,* Jianbo Li, Dermot O’Hare, Min Wei,* and Zhong Lin Wang*, Ordered-Vacancy-Induced Cation Intercalation into Layered Double Hydroxides: A General Approach for High-Performance Supercapacitors, Chem, 2018, 4, 2168–2179.

5. Wenfu Xie, Hao Li, Guoqing Cui, Jianbo Li, Yuke Song, Shijin Li, Xin Zhang, Jin Yong Lee, Mingfei Shao* and Min Wei*, NiSn Atomic Pair on Integrated Electrode for Synergistic Electrocatalytic CO2 Reduction, Angew. Chem. Int. Ed.2021, 60, 2–9.

6. Zhenhua Li, Ke Liu, Kui Fan, Yusen Yang, Mingfei Shao,* Min Wei, and Xue Duan, Active-Oxygen-Enhanced Homogeneous Nucleation of Lithium Metal on Ultrathin Layered Double Hydroxide, Angew. Chem. Int. Ed. 2019, 58, 3962–3966.

7. Lei Zhou, Mingfei Shao,* Cong Zhang, Jingwen Zhao, Shan He, Deming Rao, Min Wei,* David G. Evans, and Xue Duan, Hierarchical CoNi-Sulfide Nanosheet Arrays Derived from Layered Double Hydroxides toward Efficient Hydrazine Electrooxidation, Adv. Mater. 2017, 29, 1604080.

8. Zhenhua Li, Mingfei Shao,* Lei Zhou, Ruikang Zhang, Cong Zhang, Min Wei,* David G. Evans, Xue Duan, Directed Growth of Metal-Organic Frameworks and Their Derived Carbon-Based Network for Efficient Electrocatalytic Oxygen Reduction, Adv. Mater.2016, 28, 2337–2344.

9. Mingfei Shao, Fanyu Ning, Jingwen Zhao, Min Wei,* David G. Evans, Xue Duan, Preparation of Fe3O4@SiO2@Layered Double Hydroxide Core−Shell Microspheres for Magnetic Separation of Proteins, J. Am. Chem. Soc. 2012, 134, 1071−1077.

10. Fanyu Ning, Mingfei Shao,* Simin Xu, Yi Fu, Ruikang Zhang, Min Wei,* David G. Evans and Xue Duan, TiO2/graphene/NiFe-layered double hydroxide nanorod array photoanodes for efficient photoelectrochemical water splitting, Energy Environ. Sci. 2016, 9, 2633–2643.

11. Lan Luo†, Lingxiu Li†, Liang Xu*, Yifan Yan, Shanshan Zhang, Hua Zhou, Zhenhua Li*, Mingfei Shao*, Xue Duan, Electrosynthesis of the nylon-6 precursor from nitrate and cyclohexanone over a rutile TiO2 catalyst, CCS Chem. 2024, DOI: 10.31635/ccschem.024.202403988.

12. Lili Ma, Yucong Miao, Jiangrong Yang, Yu Fu, Yifan Yan, Zhiyuan Zhang, Zhenhua Li,* and Mingfei Shao*, Promoting Electrocatalytic Glycerol C-C Bond Cleavage to Formate Coupled with H2 Production Over a CuxNi2-xP Catalyst, Adv. Energy Mater.2024, 70, 2401061.

13. Lan Luo, Liang Xu*, Qiangyu Wang, Qiwei Shi, Hua Zhou, Zhenhua Li*, Mingfei Shao*, Xue Duan, Recent advances in external fields-enhanced electrocatalysis, Adv. Energy Mater. 2023, 13, 2301276.

14. Zhenhua Li, Xiao Zhang, Hongfei Cheng, Jiawei Liu,Mingfei Shao,* Min Wei,* David G. Evans, Hua Zhang,* and Xue Duan, Confined Synthesis of 2D Nanostructured Materials toward Electrocatalysis,Adv. Energy Mater. 2020, 10, 1900486.

15. Jianbo Li, ChunYuan Chen,Yuwei Chen, Zhenhua Li, Wenfu Xie, Xin Zhang, Mingfei Shao*and Min Wei, Polysulfide Confinement and Highly Efficient Conversion on Hierarchical Mesoporous Carbon Nanosheets for Li−S Batteries, Adv. Energy Mater. 2019, 9, 1901935.

16. Bowen Jin, Yuanhui Liu, Junya Cui, Shimeng Zhang, Yu Wu, Annan Xu, Ming Xu, Mingfei Shao*, Amorphization boost multi-ions storage for high-performance aqueous batteries, Adv. Funct. Mater. 2023, 33, 2301909.

17. Kui Fan‡, Zhenhua Li‡, Yingjie Song, Wenfu Xie, Mingfei Shao,* Min Wei*, Confinement Synthesis based on Layered Double Hydroxides: A New Strategy to Construct Single-Atom-Containing Integrated Electrodes, Adv. Funct. Mater.2021, 31, 2008064.

18. Lei Zhou, Cong Zhang, Yunqi Zhang, Zhenhua Li, and Mingfei Shao*, Host Modification of Layered Double Hydroxide Electrocatalyst to Boost the Thermodynamic and Kinetic Activity of Oxygen Evolution Reaction, Adv. Funct. Mater. 2021, 31, 2009743.

19. Wenfu Xie, Yuke Song, Shijin Li, Jianbo Li, Yusen Yang, Wei Liu, Mingfei Shao* and Min Wei*,Single-Atomic-Co Electrocatalysts with Self-Supported Architecture toward Oxygen-Involved Reaction, Adv. Funct. Mater. 2019, 29, 1906477.

20. Mingfei Shao, Fanyu Ning, Min Wei,* David G. Evans, Xue Duan,* Hierarchical Nanowire Arrays Based on ZnO Core−Layered Double Hydroxide Shell for Largely Enhanced Photoelectrochemical Water Splitting, Adv. Funct. Mater.2014, 24, 580–586.

21. Mingfei Shao, Fanyu Ning, Jingwen Zhao, Min Wei,* David G. Evans, Xue Duan, Hierarchical Layered Double Hydroxide Microspheres with Largely Enhanced Performance for Ethanol Electrooxidation, Adv. Funct. Mater.2013, 23, 3513–3518.

22. Junya Cui, Bowen Jin, Annan Xu, Jiale Li, Mingfei Shao*, Single-atom metallophilic sites for liquid NaK alloy confinement toward stable alkali-metal anodes, Adv. Sci. 2023, 2206479.

23. Qinghui Ren, Leilei Hao, Jiangrong Yang, Mengyu Lv, Hua Zhou, Zhenhua Li*, Haohong Duan*, Mingfei Shao*, Promoting electrocatalytic semihydrogenation of alkynols to alkenols over a bimetallic CuAu alloy catalyst, ACS Catal. 2024, DOI: 10.1021/acscatal.3c05928.

24. Jianbo Li, Zhenhua Li,* Fei Zhan, and Mingfei Shao*, Phase Engineering of Cobalt Hydroxide toward Cations Intercalation, Chem. Sci. 2021, 12, 1756–1761.

25. Zhenhua Li,Mingfei Shao,* Hongli An, Zixuan Wang, Simin Xu, Min Wei,* David G. Evans, Xue Duan,Fast electrosynthesis of Fe-containing layered double hydroxide arrays toward highly efficient electrocatalytic oxidation reactions Chem. Sci. 2015, 6, 6624−6631.

26. Yingjie Song, Kaiyue Ji, Haohong Duan*, Mingfei Shao*, Hydrogen production coupled with water and organic oxidation based on layered double hydroxides, Exploration 2021, 1, 20210050

27. Yucong Miao, Zhenhua Li,*, Lan Luo, Wangsong Chen, Lili Ma, Kui Fan, Yingjie Song, Yaofeng Hu, Rengui Li, Mingfei Shao*, Photoelectrocatalytic allylic C–H oxidation to allylic alcohols coupled with hydrogen evolution, Appl. Catal. B: Environ. Energy, 2025, 361, 124588

28. Yucong Miao, Zhenhua Li, Yingjie Song, Kun Fan, Jian Guo, Rengui Li, Mingfei Shao*, Surface active oxygen engineering of photoanodes to boost photoelectrochemical water and alcohol oxidation coupled with hydrogen production, Appl. Catal. B: Environ. 2023, 323, 122147.

29. Yingjie Song, Xin Wan, Yucong Miao, Jinze Li, Zhen Ren, Bowen Jin, Hua Zhou, Zhenhua Li, Mingfei Shao*, Blocking oxygen evolution reaction for efficient organic electrooxidation coupling hydrogen production by using layered double hydroxide rich in active oxygen, Appl. Catal. B: Environ. 2023, 333, 122808.

30. Yuke Song, Wenfu Xie*, Yingjie Song,Hao Li, Shijin Li, Shan Jiang, Jin Yong Lee and Mingfei Shao*, Bifunctional integrated electrode for high-efficient hydrogen production coupled with 5-Hydroxymethylfurfural oxidation, Appl. Catal. B: Environ.2022, 312, 121400.

31. Yingjie Song, Zhenhua Li, Kui Fan, Zhen Ren, Wenfu Xie, Yusen Yang, Mingfei Shao* and Min Wei, Ultrathin Layered Double Hydroxides Nanosheets Array towards Efficient Electrooxidation of 5-Hydroxymethylfurfural Coupled with Hydrogen Generation, Appl. Catal. B: Environ. 2021, 299, 120669.

32. Jingchao Liu, Si-Min Xu, Yanfei Li, Ruikang Zhang, Mingfei Shao*, Facet engineering of WO3 arrays toward highly efficient and stable photoelectrochemical hydrogen generation from natural seawater, Appl. Catal. B: Environ. 2020, 264, 118540.

33. Jingchao Liu, Jianming Li, Yanfei Li, Jian Guo, Si-Min Xu,*, Ruikang Zhang, Mingfei Shao,* Photoelectrochemical water splitting coupled with degradation of organic pollutants enhanced by surface and interface engineering of BiVO4 photoanode, Appl. Catal. B: Environ. 2020, 278, 119268.

34. Yunke Liu, Shan Jiang, Shijin Li, Lei Zhou, Zhenhua Li, Jianming Li, Mingfei Shao*,Interface engineering of (Ni, Fe)S2@MoS2 heterostructures for synergetic electrochemical water splitting, Appl. Catal. B: Environ. 2019, 247, 107–114.

35. Jinze Li, Hao Li, Kui Fan, Jin Yong Lee, Wenfu Xie*, Mingfei Shao*, Electrocatalytic nitrate reduction to ammonia coupled with organic oxidation, Chem Catal. 2023, 3, 100638.

36. ShimengZhang, YuWu, Jianxiong Gao, Yanyun Song, Bowen Jin,* MingfeiShao*, Oriented Metal Stripping for Highly Reversible Zinc Anode, Small 2024, 2402489

37. Shimeng Zhang, Jianbo Li, Bowen Jin*, Mingfei Shao*, Oriented zinc metal anode based on directional recognition and assembly, Small 2023, 19, 2301874.

38. Junya Cui, Zhenhua Li,* Annan Xu, Jianbo Li, and Mingfei Shao*, Confinement of Zinc Salt in Ultrathin Heterogeneous Film to Stabilize Zinc Metal Anode, Small 2021, 15, 2100722

39. Mingfei Shao, Zhenhua Li, Ruikang Zhang, Fanyu Ning, Min Wei,* David G. Evans, Xue Duan, Hierarchical Conducting Polymer@Clay Core–Shell Arrays for Flexible All-Solid-State Supercapacitor Devices, Small 2015, 11, 3530−3538.

40. Junya Cui, Pan Yin, Annan Xu, Bowen Jin*, Zhenhua Li, Mingfei Shao*, Fluorine Enhanced Nucleophilicity of TiO2 Nanorod Arrays: A General Approach for Dendrite-Free Anodes towards High-Performance Metal Batteries, Nano Energy 2022, 93, 106837.

41. Ruikang Zhang, Mingfei Shao,* Simin Xu, Fanyu Ning, Lei Zhou, Min Wei*, Photo-assisted synthesis of zinc-iron layered double hydroxides/TiO2 nanoarrays toward highly-efficient photoelectrochemical water splitting, Nano Energy, 2017, 33, 21–28.

42. Zhenhua Li, Mingfei Shao,* Qihui Yang, Yang Tang, Min Wei,* David G. Evans, Xue Duan, Directed Synthesis of Carbon Nanotube Arrays Based on Layered Double Hydroxides toward Highly-Efficient Bifunctional Oxygen Electrocatalysis, Nano Energy, 2017, 37, 98–107.

43. Lei Zhou, Mingfei Shao,* Jianbo Li, Shan Jiang, Min Wei,* Xue Duan, Two-Dimensional Ultrathin Arrays of CoP: Electronic Modulation toward High Performance Overall Water Splitting, Nano Energy, 2017, 41, 583–590.

44. Qihui Yang, Zhenhua Li, Ruikang Zhang, Lei Zhou, Mingfei Shao,* Min Wei, Carbon modified transition metal oxides/hydroxides nanoarrays toward high-performanceflexible all-solid-state supercapacitors, Nano Energy, 2017, 41, 408–416.

45. Zhenhua Li, Mingfei Shao,* Lei Zhou, Ruikang Zhang, Cong Zhang, Jingbin Han, Min Wei,* David G. Evans, Xue Duan, A Flexible All-Solid-State Micro-Supercapacitor Based on Hierarchical CuO@Layered Double Hydroxide Core–Shell Nanoarrays, Nano Energy 2016, 20, 294−304.

46. Zhenhua Li, Mingfei Shao,*Lei Zhou, Qihui Yang, Cong Zhang, Min Wei,* David G. Evans, Xue Duan, Carbon-based electrocatalyst derived from bimetallic metal-organic framework arrays for high performance oxygen reduction, Nano Energy 2016, 25, 100−109.

47. Chenglong Zhang, Mingfei Shao,* Fanyu Ning, Simin Xu, Zhenhua Li, Min Wei,* David G. Evans and Xue Duan,Au Nanoparticles Sensitized ZnO Nanorod@Nanoplatelet Core–Shell Arrays for Enhanced Photoelectrochemical Water Splitting, Nano Energy2015, 12, 231−239.

48. Yifan Yan†, Pengjie Hao†, Yu Fu, Wangsong Chen, Qiwei Shi, Hua Zhou, Xianggui Kong, Zhenhua Li*, Mingfei Shao*, Xue Duan. Selective electrooxidation glycerol to lactic acid coupled with hydrogen production over a cooperative BiOx/Au catalyst. AIChE J. 2024, 70, e18370.

49. Xin Du, Wenfu Xie*, Yanfei Wang, Hao Li*, Jinze Li, Yang Li, Yuke Song, Zhenhua Li, Jin Yong Lee, Mingfei Shao*, Steering benzyl alcohol electrooxidation coupled with hydrogen evolution via hetero-interface construction. AIChE J. 2024, 70, e18469

50. Wangsong Chen, Nenghui Pan, Lan Luo , Yucong Miao, Shanshan Zhang, Zhiyuan Zhang, Ruikang Zhang*, Zhenhua Li*, Mingfei Shao*. Photoelectrochemical Synthesis of Chloroprocaine from Procaine Coupled with Hydrogen Generation AIChE J. 2024, e18591

51. Jinze Li, Wenfu Xie*, Hua Zhou, Zhenhua Li, Mingfei Shao*, Techno-economic analysis of electrochemical hydrogen production coupled with alternative oxidation, Chem. Eng. Sci. 2024, 298, 120322

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